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Fractionation and Characterization of a Pine Pyrolysis Bio-Oil and In Vivo and In Silico Analysis of Its Anti-IL-17 Effects on HaCaT Human Keratinocytes
Dissertation   Open access

Fractionation and Characterization of a Pine Pyrolysis Bio-Oil and In Vivo and In Silico Analysis of Its Anti-IL-17 Effects on HaCaT Human Keratinocytes

Marwan Gagaa
Washington State University
Doctor of Philosophy (PhD), Washington State University
2023
DOI:
https://doi.org/10.7273/000006321
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Dissertation -01-03-20234.53 MBDownloadView
Open Access

Abstract

bio-oil fractionation HaCaT Human Keratinocytes psoriasis pyrolysis Adverse Effects
Psoriasis is an incurable skin disease affecting about 2-3% of the world's population. Interleukin 17 (IL-17) is a proinflammatory cytokine recognized to play a crucial role in psoriasis etiology and evolution. Monoclonal antibodies targeting IL-17A (secukinumab, ixekizumab) or its receptor (brodalumab) are available for treating psoriasis. However, their high costs, impossibility of use by topical route, and associated adverse events generate a need for identifying new anti-IL17 natural molecules. The goal of this study was to expand on earlier studies showing the beneficial effects of raw pyrolysis bio-oil on regulating IL-8 levels in keratinocytes via inhibiting IL-17. The investigation started by examining the side effects and pharmacological interactions of traditional herbal therapies for psoriasis. The bio-oil fractionation procedure was then revised and improved in the research to produce five different bio-oil fractions, each of which was characterized and put to the test on keratinocytes stimulated with IL-17. The most consistent anti-IL-17 action was seen in the aqueous fraction, which contained three pure compounds. The levels of IL-8 were effectively modulated by the mixture of two of these compounds, namely, acetic acid and acetol. According to RNA-Seq data, mitogen-activated protein kinase (MAPK) activity was found to be negatively regulated by 29 genes. This study was successful in locating effective anti-IL-17 molecules and offering details on their potential mechanisms of action.

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