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Isolation of electronic from geometric contributions to Bergman cyclization of metalloenediynes
Journal article

Isolation of electronic from geometric contributions to Bergman cyclization of metalloenediynes

Sibaprasad Bhattacharyya, Aurora E Clark, Maren Pink and Jeffrey M Zaleski
Chemical communications (Cambridge, England), Vol.9(10), pp.1156-1157
05/21/2003
Handle:
https://hdl.handle.net/2376/104806
PMID: 12778712

Abstract

Cyclization Metals - chemistry Molecular Conformation Electrochemistry Models, Molecular Diamines - chemistry Ethylenes - chemistry
Conformationally constrained ethylene-diamine metalloenediyne compounds exhibit alkyne termini separations that are constant and independent of metal center geometry. Ancillary chloride ligand electron donation into the Bergman cyclization reaction coordinate, however, dramatically influences the observed temperatures.

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